Reducing Spatial and Temporal Dimensionality in the Multidimensional Caldeira-Leggett Model

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AbstractFocusing on the real-time dynamics of the reduced density matrix of the multidimensional Caldeira-Leggett model, several techniques are adopted in this paper to reduce the spatial and temporal dimensionality, combined into an efficient algorithm. From a spatial perspective, an equivalent formulation of the Dyson series is presented. With the aid of a low-rank approximation, the spatial dimensionality of open quantum system simulations is halved. From a temporal perspective, the frozen Gaussian approximation is used to approximate both the evolution operator and the interaction operator in the multidimensional Caldeira-Leggett model. This reduces the high-dimensional integrals to one- and two-dimensional integrals independent of the truncation level of the Dyson series. Through these techniques, we design an efficient algorithm whose validity is verified through several numerical experiments, including a two-dimensional double slit simulation.Popular summaryQuantum systems are never completely isolated from their surroundings. Interactions with the environment lead to decoherence and energy dissipation, which pose key challenges for quantum technologies such as quantum computing, quantum communication, and nanoscale devices. The Caldeira-Leggett model is one of the most widely used theoretical frameworks for describing these open quantum systems. However, accurately simulating its real-time dynamics is computationally demanding because of both the high dimensionality of the system and the memory effects induced by the environment. Existing numerical approaches are therefore largely restricted to one-dimensional problems or systems with highly specialized structures. To overcome these challenges, we reduce the computational cost in two complementary ways. First, we exploit a low-rank approximation of the bath correlation function to reformulate the reduced density matrix into a representation resembling an ensemble of wavefunctions. Second, we employ the frozen Gaussian approximation, which describes quantum dynamics using Gaussian wavepackets whose centers approximate the particle motion. This provides an efficient representation of both the quantum evolution and the system-environment interaction. Consequently, the high-dimensional time integrations are reduced to only one- and two-dimensional integrals, independent of the order of the Dyson series expansion. To the best of our knowledge, this is the first deterministic algorithm capable of simulating the two-dimensional Caldeira-Leggett model. By substantially reducing both spatial and temporal complexity, our method paves the way for deterministic simulations of more realistic open systems and future numerical studies of multidimensional open quantum systems.► BibTeX data@article{Zhan2026reducingspatial, doi = {10.22331/q-2026-09-02-2201}, url = {https://doi.org/10.22331/q-2026-09-02-2201}, title = {Reducing {S}patial and {T}emporal {D}imensionality in the {M}ultidimensional {C}aldeira-{L}eggett {M}odel}, author = {Zhan, Hongfei and Pan, Ernest W.Z. and Cai, Zhenning}, journal = {{Quantum}}, issn = {2521-327X}, publisher = {{Verein zur F{\"{o}}rderung des Open Access Publizierens in den Quantenwissenschaften}}, volume = {10}, pages = {2201}, month = sep, year = {2026} }► References [1] M Grigorescu. ``Decoherence and dissipation in quantum two-state systems''. Physica A: Statistical Mechanics and its Applications 256, 149–162 (1998). https://doi.org/10.1016/S0378-4371(98)00076-4 [2] Maximilian Schlosshauer. ``Quantum decoherence''. Physics Reports 831, 1–57 (2019). https://doi.org/10.1016/j.physrep.2019.10.001 [3] Emanuel Knill and Raymond Laflamme. ``Theory of quantum error-correcting codes''. Physical Review A 55, 900 (1997). https://doi.org/10.1103/PhysRevA.55.900 [4] Michael A Nielsen and Isaac L Chuang. ``Quantum computation and quantum information''. Cambridge university press. (2010). https://doi.org/10.1017/CBO9780511976667 [5] Heinz-Peter Breuer and Francesco Petruccione. ``The theory of open quantum systems''. OUP Oxford. (2002). https://doi.org/10.1093/acprof:oso/9780199213900.001.0001 [6] Amir O Caldeira and Anthony J Leggett. ``Path integral approach to quantum brownian motion''. 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AbstractFocusing on the real-time dynamics of the reduced density matrix of the multidimensional Caldeira-Leggett model, several techniques are adopted in this paper to reduce the spatial and temporal dimensionality, combined into an efficient algorithm. From a spatial perspective, an equivalent formulation of the Dyson series is presented. With the aid of a low-rank approximation, the spatial dimensionality of open quantum system simulations is halved. From a temporal perspective, the frozen Gaussian approximation is used to approximate both the evolution operator and the interaction operator in the multidimensional Caldeira-Leggett model. This reduces the high-dimensional integrals to one- and two-dimensional integrals independent of the truncation level of the Dyson series. Through these techniques, we design an efficient algorithm whose validity is verified through several numerical experiments, including a two-dimensional double slit simulation.Popular summaryQuantum systems are never completely isolated from their surroundings. Interactions with the environment lead to decoherence and energy dissipation, which pose key challenges for quantum technologies such as quantum computing, quantum communication, and nanoscale devices. The Caldeira-Leggett model is one of the most widely used theoretical frameworks for describing these open quantum systems. However, accurately simulating its real-time dynamics is computationally demanding because of both the high dimensionality of the system and the memory effects induced by the environment. Existing numerical approaches are therefore largely restricted to one-dimensional problems or systems with highly specialized structures. To overcome these challenges, we reduce the computational cost in two complementary ways. First, we exploit a low-rank approximation of the bath correlation function to reformulate the reduced density matrix into a representation resembling an ensemble of wavefunctions. Second, we employ the frozen Gaussian approximation, which describes quantum dynamics using Gaussian wavepackets whose centers approximate the particle motion. This provides an efficient representation of both the quantum evolution and the system-environment interaction. Consequently, the high-dimensional time integrations are reduced to only one- and two-dimensional integrals, independent of the order of the Dyson series expansion. To the best of our knowledge, this is the first deterministic algorithm capable of simulating the two-dimensional Caldeira-Leggett model. By substantially reducing both spatial and temporal complexity, our method paves the way for deterministic simulations of more realistic open systems and future numerical studies of multidimensional open quantum systems.► BibTeX data@article{Zhan2026reducingspatial, doi = {10.22331/q-2026-09-02-2201}, url = {https://doi.org/10.22331/q-2026-09-02-2201}, title = {Reducing {S}patial and {T}emporal {D}imensionality in the {M}ultidimensional {C}aldeira-{L}eggett {M}odel}, author = {Zhan, Hongfei and Pan, Ernest W.Z. and Cai, Zhenning}, journal = {{Quantum}}, issn = {2521-327X}, publisher = {{Verein zur F{\"{o}}rderung des Open Access Publizierens in den Quantenwissenschaften}}, volume = {10}, pages = {2201}, month = sep, year = {2026} }► References [1] M Grigorescu. ``Decoherence and dissipation in quantum two-state systems''. Physica A: Statistical Mechanics and its Applications 256, 149–162 (1998). https://doi.org/10.1016/S0378-4371(98)00076-4 [2] Maximilian Schlosshauer. ``Quantum decoherence''. Physics Reports 831, 1–57 (2019). https://doi.org/10.1016/j.physrep.2019.10.001 [3] Emanuel Knill and Raymond Laflamme. ``Theory of quantum error-correcting codes''. Physical Review A 55, 900 (1997). https://doi.org/10.1103/PhysRevA.55.900 [4] Michael A Nielsen and Isaac L Chuang. ``Quantum computation and quantum information''. Cambridge university press. (2010). https://doi.org/10.1017/CBO9780511976667 [5] Heinz-Peter Breuer and Francesco Petruccione. ``The theory of open quantum systems''. OUP Oxford. (2002). https://doi.org/10.1093/acprof:oso/9780199213900.001.0001 [6] Amir O Caldeira and Anthony J Leggett. ``Path integral approach to quantum brownian motion''. Physica A: Statistical mechanics and its Applications 121, 587–616 (1983). https://doi.org/10.1016/0378-4371(83)90013-4 [7] David Chandler and Jerome K Percus. ``Introduction to modern statistical mechanics'' (1988). [8] Nancy Makri. ``The linear response approximation and its lowest order corrections: An influence functional approach''. The Journal of Physical Chemistry B 103, 2823–2829 (1999). https://doi.org/10.1021/jp9847540 [9] Sudip Chakravarty and Anthony J Leggett. ``Dynamics of the two-state system with ohmic dissipation''. Physical review letters 52, 5 (1984). https://doi.org/10.1103/PhysRevLett.52.5 [10] Michael Thorwart, Elisabetta Paladino, and Milena Grifoni. ``Dynamics of the spin-boson model with a structured environment''. Chemical Physics 296, 333–344 (2004). https://doi.org/10.1016/j.chemphys.2003.10.007 [11] Meng Xu and Joachim Ankerhold. ``About the performance of perturbative treatments of the spin-boson dynamics within the hierarchical equations of motion approach''.
The European Physical Journal Special Topics 232, 3209–3217 (2023). https://doi.org/10.1140/epjs/s11734-023-01000-6 [12] Nancy Makri. ``Modular path integral methodology for real-time quantum dynamics''. The Journal of Chemical Physics 149 (2018). https://doi.org/10.1063/1.5058223 [13] Geshuo Wang and Zhenning Cai. ``Real-time simulation of open quantum spin chains with the inchworm method''. Journal of Chemical Theory and Computation 19, 8523–8540 (2023). https://doi.org/10.1021/acs.jctc.3c00751 [14] Yixiao Sun, Geshuo Wang, and Zhenning Cai. ``Simulation of spin chains with off-diagonal coupling using the inchworm method''. Journal of Chemical Theory and Computation 20, 9321–9338 (2024). https://doi.org/10.1021/acs.jctc.4c00864 [15] Yaming Yan, Meng Xu, Tianchu Li, and Qiang Shi. ``Efficient propagation of the hierarchical equations of motion using the tucker and hierarchical tucker tensors''. 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