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Nonlinear Optical Quantum Communication with a Two-Dimensional Perovskite Light Source

Shuyue Feng, Zijian Gan, Camryn J. Gloor, Wei You, Andrew M. Moran
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⚡ Quantum Brief
Researchers demonstrated a novel quantum communication method using 2D organic-inorganic hybrid perovskite quantum wells, which inherently generate polarization-encoded photons without external optical manipulation. The team exploited nonlinear optical effects—specifically exciton spin dynamics and biexciton correlations—to encode information in photon ellipticity changes tracked on femtosecond timescales via four-wave mixing. They implemented the BB84 quantum key distribution protocol by mapping these intrinsic polarization states directly onto binary sequences, eliminating the need for traditional optical elements like waveplates. A 56-bit ASCII message was successfully transmitted, proving the system’s viability, with efficiency heavily dependent on biexciton state contributions and spin relaxation processes. This work highlights the potential of spin-dependent nonlinear optics in 2D perovskites for advancing integrated, material-driven quantum communication technologies.
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Quantum Physics arXiv:2511.22060 (quant-ph) [Submitted on 27 Nov 2025] Title:Nonlinear Optical Quantum Communication with a Two-Dimensional Perovskite Light Source Authors:Shuyue Feng, Zijian Gan, Camryn J. Gloor, Wei You, Andrew M. Moran View a PDF of the paper titled Nonlinear Optical Quantum Communication with a Two-Dimensional Perovskite Light Source, by Shuyue Feng and 4 other authors View PDF HTML (experimental) Abstract:Two-dimensional organic-inorganic hybrid perovskite (2D-OIHP) quantum wells are emerging as promising light sources for quantum communication technologies, owing to their ability to generate polarization-encoded optical signals. In this work, we explore how nonlinear optical phenomena can be exploited for quantum information applications, demonstrating the versatility that arises from resonant coupling among excited states. By tracking changes in the ellipticities of signal photons on femtosecond timescales in four-wave-mixing experiments, we first establish a method for information encoding based on exciton spin dynamics and biexciton correlations. Using single-photon detection, we then implement the BB84 quantum key distribution protocol by mapping these polarization states onto binary sequences. While the polarizations of weak coherent pulses are typically manipulated with optical elements in traditional quantum key distribution approaches, the intrinsic electronic structure and spin relaxation processes within the 2D-OIHP system determine the characteristics of the signal photons in our method. As a demonstration, an ASCII message consisting of 56 bits is transmitted through the polarization states of photons emitted by 2D-OIHP quantum wells. These results show that the information transmission efficiency depends strongly on contributions from biexciton states, highlighting the potential of spin-dependent nonlinear optical processes for quantum communication. Subjects: Quantum Physics (quant-ph); Chemical Physics (physics.chem-ph) Cite as: arXiv:2511.22060 [quant-ph] (or arXiv:2511.22060v1 [quant-ph] for this version) https://doi.org/10.48550/arXiv.2511.22060 Focus to learn more arXiv-issued DOI via DataCite (pending registration) Submission history From: Andrew Moran [view email] [v1] Thu, 27 Nov 2025 03:24:24 UTC (1,912 KB) Full-text links: Access Paper: View a PDF of the paper titled Nonlinear Optical Quantum Communication with a Two-Dimensional Perovskite Light Source, by Shuyue Feng and 4 other authorsView PDFHTML (experimental)TeX Source view license Current browse context: quant-ph new | recent | 2025-11 Change to browse by: physics physics.chem-ph References & Citations INSPIRE HEP NASA ADSGoogle Scholar Semantic Scholar export BibTeX citation Loading... BibTeX formatted citation × loading... Data provided by: Bookmark Bibliographic Tools Bibliographic and Citation Tools Bibliographic Explorer Toggle Bibliographic Explorer (What is the Explorer?) Connected Papers Toggle Connected Papers (What is Connected Papers?) Litmaps Toggle Litmaps (What is Litmaps?) scite.ai Toggle scite Smart Citations (What are Smart Citations?) Code, Data, Media Code, Data and Media Associated with this Article alphaXiv Toggle alphaXiv (What is alphaXiv?) Links to Code Toggle CatalyzeX Code Finder for Papers (What is CatalyzeX?) DagsHub Toggle DagsHub (What is DagsHub?) GotitPub Toggle Gotit.pub (What is GotitPub?) Huggingface Toggle Hugging Face (What is Huggingface?) Links to Code Toggle Papers with Code (What is Papers with Code?) ScienceCast Toggle ScienceCast (What is ScienceCast?) Demos Demos Replicate Toggle Replicate (What is Replicate?) Spaces Toggle Hugging Face Spaces (What is Spaces?) Spaces Toggle TXYZ.AI (What is TXYZ.AI?) Related Papers Recommenders and Search Tools Link to Influence Flower Influence Flower (What are Influence Flowers?) Core recommender toggle CORE Recommender (What is CORE?) Author Venue Institution Topic About arXivLabs arXivLabs: experimental projects with community collaborators arXivLabs is a framework that allows collaborators to develop and share new arXiv features directly on our website. Both individuals and organizations that work with arXivLabs have embraced and accepted our values of openness, community, excellence, and user data privacy. arXiv is committed to these values and only works with partners that adhere to them. Have an idea for a project that will add value for arXiv's community? Learn more about arXivLabs. Which authors of this paper are endorsers? | Disable MathJax (What is MathJax?)

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quantum-chemistry
quantum-communication
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