Towards second-long electron spin coherence of a telecom quantum emitter in naturally abundant CeO$_2$

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Quantum Physics arXiv:2605.07332 (quant-ph) [Submitted on 8 May 2026] Title:Towards second-long electron spin coherence of a telecom quantum emitter in naturally abundant CeO$_2$ Authors:Basanta Mistri, Vishal Ranjan, Siddharth Dhomkar View a PDF of the paper titled Towards second-long electron spin coherence of a telecom quantum emitter in naturally abundant CeO$_2$, by Basanta Mistri and 2 other authors View PDF HTML (experimental) Abstract:Rare-earth-ion-doped crystals has emerged as a promising platform for quantum technologies, owing to their narrow telecom-band optical emission, long spin memory, and compatibility with silicon integrated photonic architectures. However, the realization of scalable quantum devices requires host materials with intrinsically dilute spin environments to suppress decoherence. In this context, erbium (Er$^{3+}$) doped cerium oxide (CeO$_2$) is an attractive candidate due to the ultra-low concentration of nuclear spins in the host matrix and its compatibility with silicon-based technologies. Here we perform a comprehensive investigation of the coherence properties of Er$^{3+}$ electron spin qubit in CeO$_2$ via semiclassical as well as detailed cluster correlation expansion simulations. By systematically exploring magnetic field strength, pulse sequences, erbium concentration, and spin temperature, we identify regimes where decoherence from the spin bath is strongly suppressed. Our investigations illustrate that at dilute doping concentration (of the order of 10 ppb) and sub-Kelvin temperatures, operation near clock transitions enables Hahn-echo coherence times to approach the second timescale even at natural isotopic abundance. Importantly, from a practical standpoint, coherence times on the order of $\sim 10$ ms are expected even at liquid helium temperature (about 2 K) for similar concentrations. Moreover, we demonstrate that an additional enhancement can be obtained with conventional multi-$\pi$-pulse dynamical decoupling protocols. Thus, our findings establish Er$^{3+}$ doped CeO$_2$ as a front-runner for realizing spin qubits, quantum memories, and integrated quantum networks. Comments: Subjects: Quantum Physics (quant-ph) Cite as: arXiv:2605.07332 [quant-ph] (or arXiv:2605.07332v1 [quant-ph] for this version) https://doi.org/10.48550/arXiv.2605.07332 Focus to learn more arXiv-issued DOI via DataCite (pending registration) Submission history From: Basanta Mistri [view email] [v1] Fri, 8 May 2026 06:36:32 UTC (2,443 KB) Full-text links: Access Paper: View a PDF of the paper titled Towards second-long electron spin coherence of a telecom quantum emitter in naturally abundant CeO$_2$, by Basanta Mistri and 2 other authorsView PDFHTML (experimental)TeX Source view license Current browse context: quant-ph new | recent | 2026-05 References & Citations INSPIRE HEP NASA ADSGoogle Scholar Semantic Scholar export BibTeX citation Loading... BibTeX formatted citation × loading... Data provided by: Bookmark Bibliographic Tools Bibliographic and Citation Tools Bibliographic Explorer Toggle Bibliographic Explorer (What is the Explorer?) Connected Papers Toggle Connected Papers (What is Connected Papers?) Litmaps Toggle Litmaps (What is Litmaps?) scite.ai Toggle scite Smart Citations (What are Smart Citations?) Code, Data, Media Code, Data and Media Associated with this Article alphaXiv Toggle alphaXiv (What is alphaXiv?) Links to Code Toggle CatalyzeX Code Finder for Papers (What is CatalyzeX?) DagsHub Toggle DagsHub (What is DagsHub?) GotitPub Toggle Gotit.pub (What is GotitPub?) Huggingface Toggle Hugging Face (What is Huggingface?) ScienceCast Toggle ScienceCast (What is ScienceCast?) Demos Demos Replicate Toggle Replicate (What is Replicate?) Spaces Toggle Hugging Face Spaces (What is Spaces?) Spaces Toggle TXYZ.AI (What is TXYZ.AI?) Related Papers Recommenders and Search Tools Link to Influence Flower Influence Flower (What are Influence Flowers?) Core recommender toggle CORE Recommender (What is CORE?) Author Venue Institution Topic About arXivLabs arXivLabs: experimental projects with community collaborators arXivLabs is a framework that allows collaborators to develop and share new arXiv features directly on our website. Both individuals and organizations that work with arXivLabs have embraced and accepted our values of openness, community, excellence, and user data privacy. arXiv is committed to these values and only works with partners that adhere to them. Have an idea for a project that will add value for arXiv's community? Learn more about arXivLabs. Which authors of this paper are endorsers? | Disable MathJax (What is MathJax?)
